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Real and k-space microscopy of CMR manganites

One of the major challenges of contemporary physics is to gain insight into many-body problems such as high temperature superconductivity displayed by e.g. various cuprates. A similar group of materials are the manganites that display an equally poorly understood phenomenon; at the transition temperature there is a drop in resistivity of several orders of magnitude accompanied by a para- to ferromagnetic transition. This is called the colossal magnetoresistant (CMR) effect.
In the QEM group we investigate the bilayered CMR manganite La2-2xSr1+2xMn2O7 (LSMO), with various doping levels by means of angle resolved photoemission and scanning tunneling microscopy and spectroscopy. In order to do so, we use our own lab systems, the FAMoS and the Createc Ultra High Vacuum - Low Temperature (UHV-LT) STM, and synchrotron radiation provided by BESSY (Berlin, DE) and the SLS (Villigen, CH). A measurement of the Fermi surface of LSMO is shown below left as well as a typical energy distribution map in the XMY-direction. The topographic images taken on a Bi-2212 high Tc superconductor to test the STM/S system (right) show the atomic registery of the Bi atoms and characteristic incommensurate supermodulation. The single crystals measured are home-grown with an optical floating zone furnace by YingKai Huang, the crystal grower in our group.

Fermi surface of LSMO 1.) Fermi surface of LSMO EDM of LSMO in the XMY-direction
2.) EDM in the XMY-direction
Bi-2212 atomic resolution 3.) Bi-2212 (27-6-2007) Bi-2212 atomic resolution
4.) Bi-2212 (15-7-2010)

This project is the main focus of the PhD research carried out by Sanne de Jong and Freek Massee. For more information, please contact Freek Massee or Mark Golden

Results



High quality low energy electron diffraction (LEED) images of an LSMO single crystal at three different energies. Click on the image to see an IV-LEED movie ranging from 450 to 50 eV at 30K (4,51 MB).

Publications

Quasiparticles and anomalous temperature dependence of the low-lying states in the colossal
magnetoresistant oxide La2−2xSr1+2xMn2O7 (x=0.36) from angle-resolved photoemission
S. de Jong, Y. Huang, I. Santoso, F. Massee, R. Follath, O. Schwarzkopf, L. Patthey, M. Shi, and M. S. Golden
Phys. Rev. B 76 (2007) 235117 pdf (611 kB)